If you are looking to acquaint yourself with F.A. Hayek's perspective on economic theory--beyond his business cycle and monetary studies of the interwar years--this is the best source. The collection appeared in 1947, before he moved on toward broader culturaland social investigations. It contains his most profound work on the liberal economic order, and his most penetrating reflections on economic phenomena:
This is a real treasure, and the best evidence for why Hayek must be considered one of the great economists in history.
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Austrian Economics, Freedom and Peace